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We report on the benefits of changing the bridging group X of bis‐pyridyl ligands, that is, Py‐X‐Py where X is NH, CH2, C(CH3)2, or PPh, on the photo‐ and electroluminescent properties of a new family of luminescent cationic H‐heterocyclic carbene (NHC) copper(I) complexes. A joint experimental and theoretical study demonstrates that the bridging group affects the molecular conformation from a planar‐like...
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