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In the polarized infrared (IR) spectra of ordered physisorbates on insulator single crystal surfaces we observed absorption multiplets, which were assigned to correlation field or Davydov splittings, in some cases combined with site symmetry splittings. In our analysis of the infrared absorptions, based on the classical theory of dynamic dipole coupling, a two-layer model is used. The electric field...
Hydrazoic acid HN 3 molecularly adsorbed on NaCl(100) has been studied for the first time using polarization Fourier transform infrared surface spectroscopy (PIRSS) and LEED. The NaCl surface has been prepared by cleaving a single crystal in situ under UHV. Island growth up to a defined saturation coverage was observed. The strong polarization dependence of the sharp absorption multiplet of...
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