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The development of efficient and eco‐friendly methods for the synthesis of elaborate amines is highly desired as they are valuable chemicals. The catalytic alkylation of amines using alcohols as alkylating agents, through the so‐called borrowing hydrogen process, satisfies several of the principles of green chemistry. In this paper, four neutral half‐sandwich complexes of Ru(II), Rh(III), and Ir(III)...
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