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Fe3GeTe2 have proven to be of greatly intrigue. However, the underlying mechanism behind the varying Curie temperature (Tc) values remains a puzzle. This study explores the atomic structure of Fe3GeTe2 crystals exhibiting Tc values of 160, 210, and 230 K. The elemental mapping reveals a Fe‐intercalation on the interstitial sites within the van der Waals gap of the high‐Tc (210 and 230 K) samples,...
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