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Nanosecond time-resolved UV/vis absorption spectroscopy on laser flash photolysis and calculations based on (time-dependent) density functional theory for radical cations of 7-benzhydrylidenebenzonorbornene (3) and 7-benzhydrylidene-2,3-dimethylenenorbornane (4) indicated their contrasting molecular geometry and electronic structures, suggesting the nonclassical and classical nature of 3 •+ ...
Nanosecond time-resolved UV/vis absorption spectroscopy on laser flash photolysis was conducted for photoinduced electron-transfer reactions of 7-benzhydrylidenenorbornene (1) and 7-benzhydrylidenenorbornane (5). The differences in the observed absorption bands and the structures of 1 + and 5 + were evaluated successfully using calculations based on (time dependent) density functional...
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