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Efficient N2 fixation at ambient condition through electrochemical processes has been regarded as a promising alternative to traditional Haber–Bosch technology. Engineering surface atomic architecture of the catalysts to generate desirable active sites is important to facilitate electrochemical nitrogen reduction reaction (NRR) while suppressing the competitive hydrogen evolution reaction. Herein,...
In article number 2004208, Bin Li, Guangjin Zhang, and co‐workers show that by manipulation of the surface chemistry of the catalyst at the atomic level to expose Ni sites that serve as active sites for N2 reduction reaction, a novel strategy for selective exposing active facets in NiTe nanocrystal is designed. The obtained optimal catalyst shows a high Faraday efficiency of 17.38% and NH3 yield rate...
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