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Designing functional fullerenes with roles beyond defect passivation and electron‐transporting for perovskite solar cells (PSCs) is essential to the development of fullerenes and PSCs. Here, the authors design and synthesize a functional fullerene, FPD, composed of a C60 cage, a porphyrin ring, and three pentafluorophenyl groups. The structure features of FPD enable it can form chemical interactions...
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