Search results for: Sen Lin

Items from 1 to 20 out of 553 results

article

Tuning the Inter‐Metal Interaction between Ni and Fe Atoms in Dual‐Atom Catalysts to Boost CO₂ Electroreduction

Yang Chen, Jia Zhao, Xiaoli Pan, Lin Li, more

Angewandte Chemie International Edition > 63 > 44 > n/a - n/a

Dual‐atom catalysts (DACs) are promising for applications in electrochemical CO₂ reduction due to the enhanced flexibility of the catalytic sites and the synergistic effect between dual atoms. However, precisely controlling the atomic distance and identifying the dual‐atom configuration of DACs to optimize the catalytic performance remains a challenge. Here, the Ni and Fe atomic pairs were constructed...

article

Tuning the Inter‐Metal Interaction between Ni and Fe Atoms in Dual‐Atom Catalysts to Boost CO₂ Electroreduction

Yang Chen, Jia Zhao, Xiaoli Pan, Lin Li, more

Angewandte Chemie > 136 > 44 > n/a - n/a

article

Deciphering the Factors Controlling Hydrogen and Methyl Spillover upon Methane Dissociation on Rh/Cu(111) Single‐Atom Alloy

Kaixuan Gu, Hua Guo, Sen Lin

Angewandte Chemie > 136 > 39 > n/a - n/a

Spillover of adsorbed species from one active site to another is a key step in heterogeneous catalysis. However, the factors controlling this step, particularly the spillover of polyatomic species, have rarely been studied. Herein, we investigate the spillover dynamics of H* and CH₃* species on a single‐atom alloy surface (Rh/Cu(111)) upon the dissociative chemisorption of methane (CH₄), using molecular...

article

Deciphering the Factors Controlling Hydrogen and Methyl Spillover upon Methane Dissociation on Rh/Cu(111) Single‐Atom Alloy

Kaixuan Gu, Hua Guo, Sen Lin

Angewandte Chemie International Edition > 63 > 39 > n/a - n/a

article

Adsorption weakening mechanism and regulation strategy of aluminum‐based lithium adsorbents in carbonate‐style brines

Jun Chen, Jiaqi Jin, Jianguo Yu, Sen Lin

AIChE Journal > 70 > 8 > n/a - n/a

An efficient adsorption‐strengthening regulation was developed for aluminum‐based lithium adsorbents (Li/Al‐LDHs) in carbonate‐type salt lakes based on reasons for adsorption performance degradation. It was confirmed by adsorption–desorption experiments and density functional theory (DFT) that CO₃²⁻ in brines preferentially entered Li/Al‐LDH interlayers with a tighter binding energy to the laminates,...

article

In‐Situ Derived Defective Ru Particles Anchored on Ru–Ni Layered Double Hydroxides for Enhanced Alkaline Hydrogen Evolution

Ningning Shi, Ruijie Ma, Linghui Lin, Wangjing Xie, more

Small > 20 > 27 > n/a - n/a

Developing active, stable, and cost‐efficient electrocatalysts to replace platinum for the alkaline hydrogen evolution reaction (HER) is highly desirable yet represents a great challenge. Here, it is reported on a facile one‐pot synthesis of Ru_xNi layered double hydroxides (Ru_xNi‐LDHs) that exhibit remarkable HER activity and stability after an in‐situ activation treatment, surpassing most state‐of‐the‐art...

article

An ultralight all‐fiber‐structure sponge with thermal and electromagnetic integrated insulation property

Liang Su, Jiaxiang Lu, Huan Zhang, Xilin Li, more

Journal of the American Ceramic Society > 107 > 9 > 5993 - 6003

The integration of thermal and electromagnetic interference (EMI) insulation is of great significance for fields such as aerospace that face extreme environments. The challenge lies in ensuring that the protective layer is lightweight while simultaneously possessing the ability to suppress heat conduction, heat convection, thermal radiation, and electromagnetic radiation. To address these challenges,...

article

N6‐Methyladenosine reader HNRNPC‐mediated downregulation of circITCH prevents miR‐224‐3p sequestering and contributes to tumorigenesis in nasopharyngeal carcinoma

Qiang Zhou, Wei Song, Xianhui Li, Jinyan Lin, more

Environmental Toxicology > 39 > 5 > 2893 - 2907

Background N6‐Methyladenosine (m6A) RNA methylation modulators are implicated in nasopharyngeal carcinoma (NPC). Circular RNAs (circRNAs) stimulate/inhibit the development of NPC by sponging microRNAs (miRNAs). Herein, m6A modifications affecting the circRNA/miRNA axis in NPC were explored. Methods Twenty prognostic m6A RNA methylation regulators were identified from 504 head/neck squamous cell...

article

Construction of Embedded Sulfur‐Doped g‐C₃N₄/BiOBr S‐Scheme Heterojunction for Highly Efficient Visible Light Photocatalytic Degradation of Organic Compound Rhodamine B

Sen Lin, Zhangwei Sun, Xiaoyu Qiu, Han Li, more

Small > 20 > 14 > n/a - n/a

Constructing S‐scheme heterojunction catalysts is a key challenge in visible‐light catalysed degradation of organic pollutants. Most heterojunction materials are reported to face significant obstacles in the separation of photogenerated electron–hole pairs owing to differences in the material size and energy barriers. In this study, sulfur‐doped g‐C₃N₄ oxidative‐type semiconductor materials are synthesized...

article

Consolidation analysis for soft soil with non‐Darcian flow considering variable discharge capacity of prefabricated vertical drain

Zhi‐Rong Xiao, Yuan Chen, An‐Feng Hu, Sen‐Lin Xie, more

International Journal for Numerical and Analytical Methods in Geomechanics > 48 > 3 > 853 - 869

Ground improvement is a complex issue, and accurately predicting the consolidation and settlement of soft soil with prefabricated vertical drain (PVD) presents a significant challenge. Recent laboratory and field tests have highlighted the influence of the variable discharge capacity of PVD and the non‐Darcian flow behavior of soft soil on consolidation. However, existing theories have not yet considered...

article

A directional growth strategy for high layer charge Li/Al‐LDHs to reinforce Li⁺ extraction in low‐grade salt lake brines

Jun Chen, Cheng Lian, Jianguo Yu, Sen Lin

AIChE Journal > 70 > 2 > n/a - n/a

Novel Li/Al‐LDHs with high layer charges (HCLDHs) were synthesized in the light of the inter‐layer effect on Li⁺ adsorption. Compared with conventional low‐charge Li/Al‐LDHs (LCLDHs), HCLDHs exhibited a distinct micromorphology characterized by a preferential growth orientation along the c‐axis and a significantly reduced lateral diameter. Adsorption experiments showed that HCLDHs possessed superior...

article

Copper‐Catalyzed Stereoselective Defluoroalkylation or ‐arylation of gem‐Difluoroallenes To Form Monofluoroallenes under Mild Conditions

Yaoming Tan, Kailun Chen, Jiaxin Hu, Sen Lin, more

European Journal of Organic Chemistry > 27 > 2 > n/a - n/a

Herein, we demonstrate the formation of monofluoroallenes through copper‐catalyzed defluoroalkylation or defluoroarylation of gem‐difluoroallenes using affordable and readily available Grignard reagents. Additionally, alkyl lithium or alkyl zinc reagents proved successful in these transformations. Under mild conditions, monofluoroallenes can be converted into fluorinated olefinic compounds or non‐fluorinated...

article

Sustained Hydrogen Spillover on Pt/Cu(111) Single‐Atom Alloy: Dynamic Insights into Gas‐Induced Chemical Processes

Kaixuan Gu, Sen Lin

Angewandte Chemie International Edition > 62 > 47 > n/a - n/a

Hydrogen spillover, involving the surface migration of dissociated hydrogen atoms from active metal sites to the relatively inert catalyst support, plays a crucial role in hydrogen‐involved catalytic processes. However, a comprehensive understanding of how H atoms are driven to spill over from active sites onto the catalyst support is still lacking. Here, we examine the atomic‐scale perspective of...

article

Sustained Hydrogen Spillover on Pt/Cu(111) Single‐Atom Alloy: Dynamic Insights into Gas‐Induced Chemical Processes

Kaixuan Gu, Sen Lin

Angewandte Chemie > 135 > 47 > n/a - n/a

article

Why is aluminum‐based lithium adsorbent ineffective in Li⁺ extraction from sulfate‐type brines

Jun Chen, Kai Huang, Jianglong Du, Cheng Lian, more

AIChE Journal > 69 > 10 > n/a - n/a

Aluminum‐based lithium adsorbent (Li/Al‐LDH) is the only industrialized adsorbent for Li⁺ extraction from salt lake brines. The inherent mechanism of declined Li⁺ adsorption performance was revealed to explain the feebleness in sulfate‐type brines. SO₄²⁻ in brines could replace interlayer Cl⁻ by a stronger electrostatic attraction with laminates, significantly altering the stacking structure and interlayer...

article

Surface Chemistry and Catalytic Reactivity of Borocarbonitride in Oxidative Dehydrogenation of Propane

Guangming Wang, Shunhua Chen, Qiwei Duan, Fenfei Wei, more

Angewandte Chemie International Edition > 62 > 38 > n/a - n/a

Borocarbonitride (BCN) materials are newly developed oxidative dehydrogenation catalysts that can efficiently convert alkanes to alkenes. However, BCN materials tend to form bulky B₂O₃ due to over‐oxidation at the high reaction temperature, resulting in significant deactivation. Here, we report a series of super stable BCN nanosheets for the oxidative dehydrogenation of propane (ODHP) reaction. The...

article

Artificial Neuronal Devices Based on Emerging Materials: Neuronal Dynamics and Applications

Hefei Liu, Yuan Qin, Hung‐Yu Chen, Jiangbin Wu, more

Advanced Materials > 35 > 37 > n/a - n/a

Artificial neuronal devices are critical building blocks of neuromorphic computing systems and currently the subject of intense research motivated by application needs from new computing technology and more realistic brain emulation. Researchers have proposed a range of device concepts that can mimic neuronal dynamics and functions. Although the switching physics and device structures of these artificial...

article

Surface Chemistry and Catalytic Reactivity of Borocarbonitride in Oxidative Dehydrogenation of Propane

Guangming Wang, Shunhua Chen, Qiwei Duan, Fenfei Wei, more

Angewandte Chemie > 135 > 38 > n/a - n/a

article

Core‐Shell‐Type All‐Inorganic Heterometallic Nanoclusters: Record High‐Nuclearity Cobalt Polyoxoniobates for Visible‐Light‐Driven Photocatalytic CO₂ Reduction

Zheng‐Wei Guo, Ling‐Hui Lin, Jian‐Ping Ye, Yi Chen, more

Angewandte Chemie International Edition > 62 > 26 > n/a - n/a

Only rarely have polyoxometalates been found to form core–shell nanoclusters. Here, we succeeded in isolating a series of rare giant and all‐inorganic core–shell cobalt polyoxoniobates (Co−PONbs) with diverse shapes, nuclearities and original topologies, including 50‐nuclearity {Co₁₂Nb₃₈O₁₃₂}, 54‐nuclearity {Co₂₀Nb₃₄O₁₂₈}, 62‐nuclearity {Co₂₆Nb₃₆O₁₄₀} and 87‐nuclearity {Co₃₃Nb₅₄O₁₈₈}. They are the...

article

Core‐Shell‐Type All‐Inorganic Heterometallic Nanoclusters: Record High‐Nuclearity Cobalt Polyoxoniobates for Visible‐Light‐Driven Photocatalytic CO₂ Reduction

Zheng‐Wei Guo, Ling‐Hui Lin, Jian‐Ping Ye, Yi Chen, more

Angewandte Chemie > 135 > 26 > n/a - n/a

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INFONA - science communication portal

Search results for: Sen Lin

Tuning the Inter‐Metal Interaction between Ni and Fe Atoms in Dual‐Atom Catalysts to Boost CO₂ Electroreduction

Tuning the Inter‐Metal Interaction between Ni and Fe Atoms in Dual‐Atom Catalysts to Boost CO₂ Electroreduction

Deciphering the Factors Controlling Hydrogen and Methyl Spillover upon Methane Dissociation on Rh/Cu(111) Single‐Atom Alloy

Deciphering the Factors Controlling Hydrogen and Methyl Spillover upon Methane Dissociation on Rh/Cu(111) Single‐Atom Alloy

Adsorption weakening mechanism and regulation strategy of aluminum‐based lithium adsorbents in carbonate‐style brines

In‐Situ Derived Defective Ru Particles Anchored on Ru–Ni Layered Double Hydroxides for Enhanced Alkaline Hydrogen Evolution

An ultralight all‐fiber‐structure sponge with thermal and electromagnetic integrated insulation property

N6‐Methyladenosine reader HNRNPC‐mediated downregulation of circITCH prevents miR‐224‐3p sequestering and contributes to tumorigenesis in nasopharyngeal carcinoma

Construction of Embedded Sulfur‐Doped g‐C₃N₄/BiOBr S‐Scheme Heterojunction for Highly Efficient Visible Light Photocatalytic Degradation of Organic Compound Rhodamine B

Consolidation analysis for soft soil with non‐Darcian flow considering variable discharge capacity of prefabricated vertical drain

A directional growth strategy for high layer charge Li/Al‐LDHs to reinforce Li⁺ extraction in low‐grade salt lake brines

Copper‐Catalyzed Stereoselective Defluoroalkylation or ‐arylation of gem‐Difluoroallenes To Form Monofluoroallenes under Mild Conditions

Sustained Hydrogen Spillover on Pt/Cu(111) Single‐Atom Alloy: Dynamic Insights into Gas‐Induced Chemical Processes

Sustained Hydrogen Spillover on Pt/Cu(111) Single‐Atom Alloy: Dynamic Insights into Gas‐Induced Chemical Processes

Why is aluminum‐based lithium adsorbent ineffective in Li⁺ extraction from sulfate‐type brines

Surface Chemistry and Catalytic Reactivity of Borocarbonitride in Oxidative Dehydrogenation of Propane

Artificial Neuronal Devices Based on Emerging Materials: Neuronal Dynamics and Applications

Surface Chemistry and Catalytic Reactivity of Borocarbonitride in Oxidative Dehydrogenation of Propane

Core‐Shell‐Type All‐Inorganic Heterometallic Nanoclusters: Record High‐Nuclearity Cobalt Polyoxoniobates for Visible‐Light‐Driven Photocatalytic CO₂ Reduction

Core‐Shell‐Type All‐Inorganic Heterometallic Nanoclusters: Record High‐Nuclearity Cobalt Polyoxoniobates for Visible‐Light‐Driven Photocatalytic CO₂ Reduction

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