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The cover picture shows an azacalixpyridine‐supported molybdenum(0) tricarbonyl complex on gold reacting with molecular oxygen to the corresponding Mo(VI) trioxo complex which in turn catalytically mediates oxygen transfer. The reactant and the (partly gaseous) products are analyzed with a range of (surface‐) spectroscopic and analytical methods. If the carbonyl complex is irradiated (as shown in...
Adsorption of metal‐organic complexes on metallic surfaces to produce well‐defined single site catalysts is a novel approach combining the advantages of homogeneous and heterogeneous catalysis. To avoid the “surface trans‐effect” a dome‐shaped molybdenum(0) tricarbonyl complex supported by an tolylazacalix[3](2,6)pyridine ligand is synthesized. This vacuum‐evaporable complex both activates CO and...
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