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The microscopic mechanisms for higher thermoelectric performance of cost competitive rock salt compound Bi2SeS2 were investigated. A low doping of Cu as an n-type dopant was conducted in order to optimize the band structure and improve the electrical conductivity. It was revealed that this compound exhibits a Seebeck coefficient higher than 300μVK−1, which sustains above 100μVK−1 even with Cu doping,...
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