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A core feature of two‐dimensional covalent organic frameworks is crystallinity, but it remains challenging to gain their thin films with high crystallinity. Here, we presented growth of thin films of two‐dimensional covalent organic frameworks with an average domain size of ~2.83 μm2 and maximum domain size of up to ~26.19 μm2 using amphiphilic glycine derivatives on water surface. We envisage that...
Imine‐linked covalent organic frameworks (COFs) have attracted extensive attention due to designable structures, tunable properties, and excellent thermal and chemical stability. They were typically obtained as insoluble and unprocessable powders, which seriously limits their full promise. Progress has been made in the synthesis of thin films of imine‐linked COFs by interfacial synthesis. However,...
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