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Triarylboranes that exhibit p–π* conjugation serve as versatile building blocks to design n‐type organic/polymer semiconductors. A series of new molecular acceptors based on triarylborane is reported here. These molecules are designed with a boron atom that bears a bulky 2,4,6‐tri‐tert‐butylphenyl (Mes*) substituent at the core and strong electron‐withdrawing 2‐(3‐oxo‐2,3‐dihydroinden‐1‐ylidene)malononitrile...
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