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The CH bond activation of small alkanes by the gaseous MgO+. cation is probed by mass spectrometric means. In addition to H‐atom abstraction from methane, the MgO+. cation reacts with ethane, propane, n‐ and iso‐butane through several pathways, which can all be assigned to the occurrence of initial CH bond activations. Specifically, the formal CC bond cleavages observed are assigned to CH bond...
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