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Due to the narrow bandgap, environment stability, and Pt vacancy‐induced magnetism, PtSe2 has been considered a promising candidate for future broadband photodetection and electronics. However, the growth of single‐crystal PtSe2 is still a challenge. Herein, the synthesis of hexagonal and tetragonal 2H─PtSe2 single‐crystal flakes by precisely tailoring the growth temperature is reported. Through atomic...
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