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We propose a new predictive approach for the calculation of properties and phase behavior of mixtures containing ionic liquids (ILs). In this method the Pitzer–Debye–Hückel (PDH) model for the long-range electrostatic interactions is combined with the COSMO-SAC model for the short-range interactions between contacting molecules. While the COSMO-SAC model alone has been shown to be accurate for vapor–liquid...
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