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Stable battery operation involving high‐capacity electrode materials such as tin (Sn) has been plagued by dimensional instability‐driven battery degradation despite the potentially accessible high energy density of batteries. Rational design of Sn‐based electrodes inevitably requires buffering or passivation layers mostly in a multi‐stacked manner with sufficient void inside the shells. However, undesirable...
In article number 2004861, Soojin Park, Hyunjung Lee, and co‐workers present an inverse design for high‐capacity Sn anodes that ensures the structural stability of three‐dimensional freestanding electrodes as incorporated with dual buffers. Outmost TiO2 nanoshells as a mechanically stable passivation layer allow for inward reversible breathing of Sn anodes while macroporous rGO framework provides...
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