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Undercoordination chemistry is an effective strategy to modulate the geometry‐governed electronic structure and thereby regulate the activity of sulfur electrocatalysts. Efficient sulfur electrocatalysis is requisite to overcome the sluggish kinetics in lithium–sulfur (Li–S) batteries aroused by multi‐electron transfer and multi‐phase conversions. Recent advances unveil the great promise of undercoordination...
Described herein presents a kind of multisite hybrid ionic liquid‐catalysts and establishes a novel strategy for H2S utilization, which has been characterized by multiaspects to reveal internal structural characterization. Through chemical modification, the D101‐based hybrid ILs were used for the direct synthesis of thioamides from the addition of H2S and nitriles. D101‐[PMDETA][DMG] can achieve an...