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The development of efficient photodetectors (PDs) for ultraviolet (UV) light is of great importance for many applications. In this paper, a novel approach is proposed for boosting the performances of self‐powered PDs. Visible‐blind UV‐A PDs are built by combining a mesoporous TiO2 layer with a Spiro‐OMeTAD layer. The nanostructured heterointerface is engineered by inserting a self‐assembled layer...
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