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Donor substituted heteroleptic bis-tridentate Ru(II) complexes with different deprotonated forms exhibit larger alterations of the first hyperpolarizabilities in oxidized process and are promising to become redox-switchable nonlinear optical (NLO) molecular materials. For systems with diprotonated form, the β vec value of the two-electron-oxidized system 1 3 2+ is 5.3 and 178...
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