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The electrochemical carbon dioxide reduction reaction (CO2RR) to formate is of great interest in the field of electrochemical energy. Cu‐based material is an appealing electrocatalyst for the CO2RR. However, retaining Cu2+ under the high cathodic potential of CO2RR remains a great challenge, leading to low electrocatalytic selectivity, activity, and stability. Herein, inspired by corrosion science,...