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Optoelectronic applications of organic semiconductors demand single‐crystalline structures with long‐range order and suppressed defects for sustaining efficient carrier transport and long photocarrier lifetime, which are pivotal in photodetection, photovoltaic, and light emission. For integrated devices, an additional requirement of precise patterning is imposed, whereas the patterning of single‐crystalline...
All‐inorganic metal‐halide perovskites CsPbX3 (X = Cl, Br, I) exhibit higher stability than their organic–inorganic hybrid counterparts, but the thermodynamically instable perovskite α phase at room temperature of CsPbI3 restricts the practical optoelectronic applications. Although the stabilization of α‐CsPbI3 polycrystalline thin films is extensively studied, the creation of highly crystalline micro/nanostructures...
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