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This work presents a DFT‐based computational study on the regio‐ and enantioselective C−H functionalization of pyridines with alkenes at the relatively unreactive C4‐position, which was successfully achieved by Shi et al. [J. Am. Chem. Soc. 2019, 141, 5628–5634] using Ni0/N‐heterocyclic carbene (NHC) catalysis under the assistance of an aluminum‐based Lewis acid additive (2,6‐tBu2‐4‐Me‐C6H2O)2AlMe...
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