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The effect of vibrational excitation, for example by infrared (IR) laser pulses, on the photodesorption of H 2 and D 2 from a Ru(0001) surface has been investigated theoretically. Based on information from first principle electronic structure theory, a minimal two-mode and two-state model is developed for Desorption Induced by Electronic Transitions (DIET) in the single-excitation...
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