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Ceramics with perovskite structure and composition BaCexTi1−xO3 (x = 0.02–0.30) show a progressive evolution with increasing x, from the long‐range polar order of ferroelectric BaTiO3 to the short‐range polar order typical of relaxors. The ionic size mismatch between Ti4+ and Ce4+ determines strong local strains which have a significant impact on dielectric properties and phase transitions. The pair...
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