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A cytosine-substituted nitronyl nitroxide monoradical 1 and a biradical 2 with a singlet (S=0) ground state have been synthesized and characterized as building blocks for organic molecule-based magnets. X-ray crystallographic analyses have shown that the molecular packing of 1 features in intermolecular hydrogen bonding of the cytosine moiety, giving a spin ladder chain structure based on nitronyl...
A novel iminonitroxide triradical, p-triIN (1), has been synthesized, in which a π-conjugated biradical with a singlet ground state and a doublet monoradical are united by σ-bonds. The intramolecular exchange interaction within the para-phenylene-based biradical moiety has been found to be antiferromagnetic (2J(π)/k B =−30.8K) from magnetic susceptibility measurements on a parent biradical,...
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