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The dense, anhydrous zeolitic imidazolate frameworks (ZIFs), Zn(Im)2 (1) and LiB(Im)4 (2), adopt the same zni topology and differ only in terms of the inorganic species present in their structures. Their mechanical properties (specifically the Young’s and bulk moduli, along with the hardness) have been elucidated by using high pressure, synchrotron X‐ray diffraction, density functional calculations...
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