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We investigated the oxidation of Ir(111) by gas-phase oxygen atoms at temperatures between 500 and 625K using temperature programmed desorption (TPD), low energy electron diffraction (LEED), low energy ion scattering spectroscopy (LEISS) and density functional theory (DFT) calculations. We find that a well-ordered surface oxide with (√3×√3)R30° periodicity relative to Ir(111) develops prior to the...
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