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The asymmetric C‐alkylation of chiral enamines derived from terminal epoxides and lithium 2,2,6‐trialkylpiperidides has previously been shown to provide α‐alkylated aldehydes by intermolecular nucleophilic substitution in good levels of asymmetric induction. We now report a computational study of the origins of asymmetric induction in these reactions. Computational modeling with density functional...
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