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Reactions of N,N‐dimethylaniline (DMA) with nonheme iron(IV)‐oxo and iron(IV)‐tosylimido complexes occur via different mechanisms, such as an N‐demethylation of DMA by a nonheme iron(IV)‐oxo complex or an electron transfer dimerization of DMA by a nonheme iron(IV)‐tosylimido complex. The change in the reaction mechanism results from the greatly enhanced electron transfer reactivity of the iron(IV)‐tosylimido...
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