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The rational design of catalytically active sites in porous materials is essential in electrocatalysis. Herein, atomically dispersed Fe‐Nx sites supported by hierarchically porous carbon membranes are designed to electrocatalyze the hydrazine oxidation reaction (HzOR), one of the key techniques in electrochemical nitrogen transformation. The high intrinsic catalytic activity of the Fe‐Nx single‐atom...
In article number 2002203, Tian Sheng, Shu‐Hui Sun, Jiayin Yuan, and co‐workers propose and verify atomically dispersed pyrrole‐type Fe‐N4 sites supported on hierarchically porous carbon membranes as real active sites for the electrochemical hydrazine oxidation reaction (HzOR), which will open up the future exploration of the metal‐Nx catalysts for HzOR in fuel cells and beyond.
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