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We report the synthesis of higher-molecular-weight hyperbranched polyethylenes containing cross-linking structures via chain walking copolymerization of ethylene with a diacrylate cross-linker, 1,4-butanediol diacrylate, using a Pd-diimine catalyst, [(ArNC(Me)–(Me)CNAr)Pd(CH 3 )(NCMe)]SbF 6 (Ar=2,6-(iPr) 2 C 6 H 3 ). The hyperbranched chain topology of these...
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