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Two azide‐bridged coordination polymers, [Cu(mptz)(N3)2] (1) and [Mn(mptz)(N3)2H2O] (2), (mptz = N‐methyl‐4‐pyridinium tetrazolate), were synthesized and crystallographically and magnetically characterized. Compound 1 is a neutral 1D coordination polymer in which the CuII ions, which are in a square pyramidal surrounding, are linked by double end‐on azide bridges in an alternating basal–basal and...
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