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The bulk and surface of a perovskite light‐harvesting layer are two pivotal aspects affecting its carrier transport and long‐term stability. In this work, lead(II) 2‐ethylhexanoate (LDE) is introduced via an antisolvent process into perovskite films to change the reaction kinetics of the crystallization process, resulting in a high‐quality perovskite film. Meanwhile, a carboxyl functional group with...
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