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A radical change: Two 3D ZnII complexes with pillared structures have been synthesized from a triamine‐based polycarboxylate ligand under hydrothermal conditions. The complexes exhibit reversible radical‐based redox photochromism that varies from yellow to bluish‐violet and dark blue, respectively, under UV/blue irradiation, and fluorescence with adjustable intensity. The ESR and X‐ray photoelectron...
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