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A cesium bismuth germanate, Cs2Bi2O(Ge2O7) (CBGO), was synthesized by a traditional high‐temperature solid‐state reaction. Its structure features a 3D network composed of a 1D chains composed of Bi2O8 dimers that are further bridged by Ge2O7 dimers, forming tunnels of seven member rings (MRs) that are filled by the Cs+ cations. CBGO exhibits extraordinary larger second harmonic generation (SHG) response...
The first metal iodate fluoride, Bi(IO3)F2, with a strong second harmonic generation (SHG) effect has been prepared. Bi(IO3)F2 crystallizes in the polar space group C2 and features a three‐dimensional [BiF2]+ cationic framework with IO3 groups capping the inner walls of the one‐dimensional tunnels. This [BiF2]+ cationic framework acts as a template for the assembly of the polar IO3 units in a favorable...
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