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Bridging iron hydrides are proposed to form at the active site of MoFe‐nitrogenase during catalytic dinitrogen reduction to ammonia and may be key in the binding and activation of N2 via reductive elimination of H2. This possibility inspires the investigation of well‐defined molecular iron hydrides as precursors for catalytic N2‐to‐NH3 conversion. Herein, we describe the synthesis and characterization...
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