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Co‐crystallization of a cyanide‐bridged tetranuclear complex [Co2Fe2] with 4‐cyanophenol (CP) gave a hydrogen bonding donor–acceptor system, [Co2Fe2(bpy*)4(CN)6(tp*)2](PF6)2⋅2 CP⋅8 BN (1). 1 exhibited a three‐step phase transition between HT, IM1, IM2, and LT phases upon temperature variation. Variable temperature magnetic measurements and structural analyses revealed that the three‐step spin transition...
Dynamische Wasserstoffbrücken‐Wechselwirkungen …… gekoppelt mit Spinübergangsverhalten spielen eine wichtige Rolle für die Stabilisierung von Zwischenphasen in einem mehrstufigen Spinübergang. In ihrer Zuschrift auf S. 606 ff. stellen M. Nihei, H. Oshio et al. ein wasserstoffverbrücktes Donor‐Akzeptor‐System vor, das aus einem spinübergangsaktiven quadratischen [Co2Fe2]‐Komplex und aromatischen Wasserstoffbrücken‐Donormolekülen...
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