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Exploring TiO2‐photocatalysts for sunlight conversion has high demand in artificial photosynthesis. In this work, edge‐enriched ultrathin molybdenum disulfide (MoS2) flakes are uniformly embedded into the bulk of yolk‐shell TiO2 as a cocatalyst to accelerate photogenerated‐electron transfer from the bulk to the surface of TiO2. The as‐formed MoS2/TiO2 (0.14 wt%) hybrids exhibit a high hydrogen evolution...
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