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High‐valent iron: The electronic structures of [FeIII(Et2dtc)3−n(mnt)n]n− (mnt=maleonitriledithiolate and Et2dtc=diethyldithiocarbamato; n=3, 2, 1, 0) and their one‐electron oxidized analogues have been elucidated and correlated with the structural and spectroscopic parameters of the complexes (see figure). Despite the presence of noninnocent dithiolene ligands, the oxidized complexes are best described...
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