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3D and 2D hybrid perovskites, which have been known for more than 20 years, have emerged recently as promising materials for optoelectronic applications, particularly the 3D compound (CH3NH3)PbI3 (MAPI). The discovery of a new family of hybrid perovskites called d‐MAPI is reported: the association of PbI2 with both methyl ammonium (MA+) and hydroxyethyl ammonium (HEA+) cations leads to a series of...
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