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In elektrokatalytischen CO2‐Systemen können die Solvatisierung von Zwischenstufen durch Wasser und ihre Wechselwirkungen auf Katalysatoroberflächen die Leistung einschneidend verändern. W. Smith und Mitarbeiter zeigen in ihrer Zuschrift auf S. 1359, dass *OCHO, eine Zwischenstufe der Formiatbildung, leicht auf der Oberfläche hauptsächlich CO erzeugender Katalysatoren wie Ag gebildet werden kann. *OCHO...
Ag is a promising catalyst for the production of carbon monoxide (CO) via the electrochemical reduction of carbon dioxide (CO2ER). Herein, we study the role of the formate (HCOO−) intermediate *OCHO, aiming to resolve the discrepancy between the theoretical understanding and experimental performance of Ag. We show that the first coupled proton‐electron transfer (CPET) step in the CO pathway competes...
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