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A cationic metal–organic framework (MOF), [Cu2L(H2O)2]⋅(NO3)2⋅5.5 H2O (1) has been successfully synthesized from a zwitterionic ligand 1,1′‐bis(3,5‐dicarboxyphenyl)‐4,4′‐bipyridinium chlorine ([H4L]Cl2). The framework of compound 1 contains classical {Cu2(O2C)4} paddlewheels, and possesses typical nbo‐type topology and two types of channels with sizes of 5.0 and 15.54 Å. Benefitting from the 3D cationic...
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