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Photo-healable ion gels with improved mechanical properties are demonstrated using a tetra-arm diblock copolymer (A(B)4) containing azobenzene groups. Physical ion gels were prepared by self-assembly of A(B)4 in a hydrophobic ionic liquid, 1-butyl-3-methylimidazolium hexafluorophosphate ([C4mim]PF6), where A block is the ionic liquid-compatible tetra-PEG, and B block is the thermo-/photo-responsive...
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