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The catalytic hydrodeoxygenation of C 3 alcohols (1- and 2-propanol, 1,2- and 1,3-propanediol, and glycerol) on Pt/Al 2 O 3 has been mechanistically explored in the aqueous phase. Dehydrogenation on Pt and dehydration on alumina are the main elementary reaction pathways. In water, carbon–carbon bond cleavage for alcohols with terminal hydroxyl groups occurs via decarbonylation...
The oxidation state and the structural properties of Al2O3-supported bimetallic PdCu catalysts during the catalytic reduction of KNO3 carried out in the aqueous phase were investigated by X-ray absorption spectroscopy. Under reaction conditions the noble metal component (Pd) was in a reduced state, while the less noble metal (Cu) was found to be partially oxidized. A PdCu phase was formed in the bimetallic...
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