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A solid‐state battery with a lithium‐metal anode and a garnet‐type solid electrolyte has been widely regarded as one of the most promising solutions to boost the safety and energy density of current lithium‐ion batteries. However, lithiophobic property of garnet‐type solid electrolytes hinders the establishment of a good physical contact with lithium metal, bringing about a large lithium/garnet interfacial...
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