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Massive efforts have been devoted to designing molecular ferroic materials by molecular modification. For molecular ferroelastic, previous work is focused on the temperature‐dependent ferroelastic domains, however, few are related to controlling the ferroelastic domain by the stress. Inspired by the “quasi‐spherical theory” and fluorination effect, we designed a more flexible (MedabcoF)2+ (MedabcoF=1‐fluoro‐4‐methyl‐1,4‐diazoniabicyclo[2...
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