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Low conductivity over a wide temperature region due to ultra‐slow ion migration dynamics is a key issue in the field of solid‐state electrolytes (SSE), which needs to be solved and improved. Covalent organic frameworks (COFs), a rapidly growing class of porous crystalline materials, emerge as a new research hotspot in the field of SSEs. This is due to their homogeneously dispersed sites and well‐defined...
A novel kind of solid‐state lithium electrolyte was fabricated by impregnating organic ionic plastic crystals (OIPCs) into the pores of covalent organic frameworks (COFs). The liquid‐like phase of confined N,N‐dimethylpyrrolidinium iodide (P1,1I) and the ordered nanochannels of COFs simultaneously stimulated the lithium ion conduction.
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