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Reduction of ferredoxin by photosystem I (PSI) involves the [4Fe–4S] clusters FA and FB harbored by PsaC, with FB being the direct electron transfer partner of ferredoxin (Fd). Binding of the redox-inactive gallium ferredoxin to PSI was investigated by flash-absorption spectroscopy, studying both the P700+ decay and the reduction of the native iron Fd in the presence of FdGa. FdGa binding resulted...
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