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Light‐driven CO2 reduction into high value‐added product is a potential route to convert and store solar energy. Here, using the hydroxyls on an oxyhydroxide photocatalyst, CoGeO2(OH)2, as solid‐state proton source to reduce the CO2 into CH4 is proposed. It is found that under irradiation, the lattice hydroxyls on surface of CoGeO2(OH)2 are oxidized by photogenerated holes, resulting in the generation...
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