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We present here a new photoelectrochemical method for varying the pH locally to trigger silica condensation at the interface between two immiscible electrolyte solutions (ITIES). Trimethylbenzhydrylammonium cation is a photoactive compound dissolved in the organic phase. Electrochemical studies have shown a reversible transfer across the interface controlled by diffusion. Its transfer from the organic...
In this work, the array of miniaturized interfaces between two immiscible electrolyte solutions was modified with a mesoporous silica material. The electrochemical behavior of such silica deposits was evaluated with six analytes: 3 tetraalkylammonium cations of different sizes, the anionic 4-octylbenzenesulfonate and two poly(aminoamide) dendrimers (generation 0 and 1). Presence of silica deposits...
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